unstrap

[uhn-strap]
verb (used with object), unstrapped, unstrapping.
to take off or slacken the strap of.

Origin:
1820–30; un-2 + strap

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Based on the Random House Dictionary, © Random House, Inc. 2014.
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WordNet
unstrap

verb
remove the strap or straps from [ant: strap
WordNet® 3.0, © 2006 by Princeton University.
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Example sentences
Some struggled to unstrap their seat belts as smoke began to fill the cabin.
It would be much simpler and better to unstrap his fettered leg.
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