bound by or as if by a spell; enchanted, entranced, or fascinated: a spellbound audience.

1790–1800; spell2 + -bound1

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verb (used with object), spellbound, spellbinding.
to hold or bind by or as if by a spell; enchant; entrance; fascinate.

1800–10; spell2 + bind, deduced from spellbound

spellbindingly, adverb
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Based on the Random House Dictionary, © Random House, Inc. 2014.
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World English Dictionary
spellbind (ˈspɛlˌbaɪnd)
vb , -binds, -binding, -bound
(tr) to cause to be spellbound; entrance or enthral

spellbound (ˈspɛlˌbaʊnd)
having one's attention held as though one is bound by a spell: a spellbound audience

Collins English Dictionary - Complete & Unabridged 10th Edition
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Example sentences
But even those who did not were held spellbound by the swinging sonorous
He can spin a tale, keep the poem going through countless twists and turns of
  the plot, and hold us spellbound.
Even aged and nearly mute, pop's great bombshell could hold an audience
Many visitors have been spellbound while watching the daily activities of the
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